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Highly ordered graphite (HOPG) to hexagonal diamond (lonsdaleite) phase transition observed on picosecond time scales using ultrafast x-ray diffraction

Urheber*innen

Armstrong,  Michael R.
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Radousky,  Harry B.
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Austin,  Ryan A.
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Tschauner,  Oliver
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Brown,  Shaughnessy
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Gleason,  Arianna E.
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Goldman,  Nir
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Granados,  Eduardo
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Grivickas,  Paulius
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Holtgrewe,  Nicholas
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Kroonblawd,  Matthew P.
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Lee,  Hae Ja
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/persons/resource/slobanov

Lobanov,  S. S.
0 Pre-GFZ, Departments, GFZ Publication Database, Deutsches GeoForschungsZentrum;

Nagler,  Bob
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Nam,  Inhyuk
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Prakapenka,  Vitali
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Prescher,  Clemens
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Reed,  Evan J.
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Stavrou,  Elissaios
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Walter,  Peter
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Goncharov,  Alexander F.
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Belof,  Jonathan L.
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Zitation

Armstrong, M. R., Radousky, H. B., Austin, R. A., Tschauner, O., Brown, S., Gleason, A. E., Goldman, N., Granados, E., Grivickas, P., Holtgrewe, N., Kroonblawd, M. P., Lee, H. J., Lobanov, S. S., Nagler, B., Nam, I., Prakapenka, V., Prescher, C., Reed, E. J., Stavrou, E., Walter, P., Goncharov, A. F., Belof, J. L. (2022): Highly ordered graphite (HOPG) to hexagonal diamond (lonsdaleite) phase transition observed on picosecond time scales using ultrafast x-ray diffraction. - Journal of Applied Physics, 132, 5, 055901.
https://doi.org/10.1063/5.0085297


Zitierlink: https://gfzpublic.gfz-potsdam.de/pubman/item/item_5012716
Zusammenfassung
The response of rapidly compressed highly oriented pyrolytic graphite (HOPG) normal to its basal plane was investigated at a pressure of ∼80 GPa. Ultrafast x-ray diffraction using ∼100 fs pulses at the Materials Under Extreme Conditions sector of the Linac Coherent Light Source was used to probe the changes in crystal structure resulting from picosecond timescale compression at laser drive energies ranging from 2.5 to 250 mJ. A phase transformation from HOPG to a highly textured hexagonal diamond structure is observed at the highest energy, followed by relaxation to a still highly oriented, but distorted graphite structure following release. We observe the formation of a highly oriented lonsdaleite within 20 ps, subsequent to compression. This suggests that a diffusionless martensitic mechanism may play a fundamental role in phase transition, as speculated in an early work on this system, and more recent static studies of diamonds formed in impact events.